Proton permselective solid-state member and apparatus utilizing said permselective member
First Claim
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1. A proton permselective solid-state member, formed by shaping at least one member selected from the group consisting of heteropoly acids represented by the generic formula:
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space="preserve" listing-type="equation">H.sub.m [X.sub.x Y.sub.y O.sub.z ].sup.. nH.sub.2 Owherein, X stands for at least one member selected from the group consisting of boron, aluminum, gallium, silicon, germanium, tin, phosphorus, arsenic, antimony, bismuth, selenium, tellurium, iodine and transition metals belonging to the fourth, fifth and sixth periods of the Periodic Table, Y is at least one member selected from transition metals belonging to the fourth, fifth, and sixth periods of the Periodic Table, and wherein m has a value of from 2 to 10, y has a value of from 1 to 12, n has a value of from 3 to 100 all based on X taken as 1 and z has a positive numerical value and salts of said acids.
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Abstract
Disclosed is a proton permselective solid-state member which is formed of a heteropoly acid represented by the generic formula, Hm [Xx.sup.. Yy.sup.. Oz ].sup.. nH2 O, or a salt thereof. Said permselective member can be used as an electrolyte in the fuel cell and as a permselective membrane in the hydrogen gas refining system.
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Citations
13 Claims
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1. A proton permselective solid-state member, formed by shaping at least one member selected from the group consisting of heteropoly acids represented by the generic formula:
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space="preserve" listing-type="equation">H.sub.m [X.sub.x Y.sub.y O.sub.z ].sup.. nH.sub.2 Owherein, X stands for at least one member selected from the group consisting of boron, aluminum, gallium, silicon, germanium, tin, phosphorus, arsenic, antimony, bismuth, selenium, tellurium, iodine and transition metals belonging to the fourth, fifth and sixth periods of the Periodic Table, Y is at least one member selected from transition metals belonging to the fourth, fifth, and sixth periods of the Periodic Table, and wherein m has a value of from 2 to 10, y has a value of from 1 to 12, n has a value of from 3 to 100 all based on X taken as 1 and z has a positive numerical value and salts of said acids. - View Dependent Claims (2, 3, 4, 5)
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6. An apparatus having an anode chamber and a cathode chamber separated from each other by a partition wall provided with catalysts and leading wires on the surfaces thereof facing said anode and cathod chambers, said partition wall being an article obtained by shaping at least one member selected from the group consisting of heteropoly acids represented by the generic formula:
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space="preserve" listing-type="equation">H.sub.m [X.sub.x Y.sub.y O.sub.z ].sup.. nH.sub.2 Owherein, X stands for at least one member selected from the group consisting of boron, aluminum, gallium, silicon, germanium, tin, phosphorus, arsenic, antimony, bismuth, selenium, tellurium, iodine and transition metals belonging to the fourth, fifth and sixth periods of the Periodic Table, Y for at least one member selected from transition metals belonging to the fourth, fifth and sixth periods of the Periodic Table, and wherein m has a value of from 2 to 10, y has a value of from 1 to 12, n has a value of from 3 to 100, all based on X as taken 1 and z has a positive numerical value and salts of said acids. - View Dependent Claims (7, 8, 9, 10, 11, 12, 13)
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Specification