Detection of nitrogen in explosives

• US 4,851,687 A
• Filed: 01/13/1987
• Issued: 07/25/1989
• Est. Priority Date: 01/13/1987
• Status: Expired due to Term

• Current Assignee: Scientific Food Solutions, LLC
• Original Assignee: Scientific Food Solutions, LLC
• Inventors: Brondo, Joseph H. Jr., Ettinger, Kamil V.
• Primary Examiner(s): Howell, Janice A.
• Assistant Examiner(s): NOT, DEFINED
• Application Number:
  US07/002,788
• Time in Patent Office: 924 Days
• Field of Search: 250/390 C, 250/252.1, 250/390 R, 250/354.1, 250/370 C, 250/370 I, 250/370 J, 250/370 K, 250/367, 376/158, 376/159
• US Class Current: 250/390.04
• CPC Class Codes: G01V 5/234 Measuring induced radiation, e.g. thermal neutron activation analysis

Abstract

An apparatus and method for scanning an object for nitrogen for detecting the presence of explosives in luggage, parcels and the like. The object is placed in a cavity in which a thermal neutron flux is produced by introducing fast neutrons in the presence of a nuclear moderating material. A reaction between the thermal neutrons and the nitrogen contained in the object causes gamma rays to be emitted which are detected and transmitted to processing electronics to determine the concentration and position of nitrogen in the object. Thermal neutrons sensors are located within the cavity to monitor the amount of thermal neutrons and adjust the thermal neutron flux within the cavity in order to maintain an optimal thermal neutron flux density within the cavity. The adjustment may be effectuated by adjusting the accelerating potential of a neutron accelerator or by adjusting the position of a neutron moderator for use with an isotopic neutron source.

Claims

1. An apparatus for scanning an object to determine the concentration and position of nitrogen in the object comprising:

a housing having a cavity for receiving an object to be scanned and means for passing the object through said cavity;

means for producing a thermal neutron flux within said cavity, said thermal neutron flux causing high energy gamma rays to be emitted from said object as the object passes through said cavity in response to reactions with nitrogen contained in said object;

means for sensing the amount of thermal neutrons within said cavity;

means for adjusting the thermal neutron flux within said cavity in response to the amount of thermal neutrons to maintain a predetermined thermal neutron flux density within said cavity;

at least one primary radiation detector within the cavity for detecting the high energy gamma rays emitted by the object as the object passes said radiation detector(s) and for producing output signals representative of the position and energy of said gamma rays; and

means for processing and analyzing said output signals for determining the concentration and position of nitrogen in said object.

2. The apparatus of claim 1, wherein said means for producing a thermal neutron flux includes a fast neutron source.

3. The apparatus of claim 2 wherein said means for sensing the amount of thermal neutrons includes at least one neutron flux sensor that produces electrical output signals representative of the amount of thermal neutrons within said cavity.

4. The apparatus of claim 3 wherein said means for adjusting the thermal neutron flux includes an amplifier and a rate counter coupled to each of said flux sensors for counting the electrical output signals, and a computer control means for determining the cavity thermal neutron flux density, said computer control means producing a control signal to adjust the thermal neutron flux within the cavity in response to the amount of thermal neutrons within said cavity.

5. The apparatus of claim 4 wherein said means for sensing the amount of thermal neutrons is located within said cavity in a position to minimize detection of fast neutrons.

6. The apparatus of claim 4 wherein said means for adjusting the thermal neutron flux includes a reference value memory means that inputs a reference signal representative of the predetermined neutron flux density into said computer control means for comparison with the cavity thermal neutron density determined from the amount of thermal neutrons inputted to said computer control means from said counters, said computer control means producing the control signal in response to a difference between the predetermined thermal neutron flux density and the cavity thermal neutron flux density.

7. The apparatus of claim 6 wherein said means for producing a thermal neutron flux further includes a neutron collimator having a passage for directing a beam of fast neutrons into an irradiation zone within said cavity.

8. The apparatus of claim 7 wherein said fast neutron source is an accelerator and the control signal from said computer control means adjusts the accelerating potential of said accelerator thereby adjusting the thermal neutron flux with said cavity.

9. The apparatus of claim 7 wherein said fast neutron source is an isotopic source.

10. The apparatus of claims 8 or 9 wherein said means for producing a thermal neutron flux further includes a neutron moderator movably alignable with the passage of said neutron collimator to be selectively within the beam of fast neutrons.

11. The apparatus of claim 10 further including means for selectively moving said neutron moderator within the beam of fast neutrons in response to the control signal from said computer control means.

12. The apparatus of claim 11 further including a switch means for selectively coupling said control signal to said means for moving said neutron moderator and said accelerator.

13. The apparatus of claim 6 wherein said housing includes a conveyor means for introducing said object to be scanned into said housing to pass said object through said irradiation zone.

14. The apparatus of claim 13 wherein said conveyor means is transparent to both neutrons and gamma rays.

15. The apparatus of claim 14 wherein said housing includes an inner lining of a neutron moderator material.

16. The apparatus of claim 15 wherein said housing is located within an outer enclosure and said conveyor means introduces the object first into said outer enclosure and second into said housing.

17. The apparatus of claim 1 wherein said means for analyzing said output signals includes means for providing an image of the nitrogen distribution contained within the object.

18. The apparatus of claim 1 wherein said means for analyzing said output signals includes register means for addressing the output signals from said detector(s) in accordance with a timing pulse thereby storing information representative of a plurality of discrete portions of object as the object passes said detector(s).

19. The apparatus of claim 18 wherein said radiation detector includes a conversion foil for converting the gamma rays into electrons, an electron collimator having a plurality of channels with openings on opposed sides of said collimator for receiving said converted electrons, said conversion foil being secured to said collimator to cover the openings on one side of said collimator, and an array of electron scintillators each coupled to a photomultiplier arranged to detect the electrons passing through each of said channels and to provide output signals representative of the position and concentration of nitrogen contained in said object.

20. The apparatus of claim 18 wherein said radiation detector includes a conversion foil for converting gamma rays into electrons, a channeling crystal coupled to said conversion foil for producing channeling radiation in response to electrons travelling through said crystal substantially parallel to the plane of the crystal lattice, an electron detector for producing first signals in response to electrons passing through said crystal lattice and a solid state channeling radiation detector for producing second signals representative of the position and concentration of nitrogen contained in the object.

21. The apparatus of claim 20 wherein said means for analyzing said output signals includes a coincidence circuit coupled to receive the signals from the electron detector and the channeling radiation detector for producing an output signal to said register only upon outputs being received from both the electron detector and the channeling detector.

22. The apparatus of claim 20 wherein said electron detector is a semiconductor surface barrier detector.

23. The apparatus of claim 20 wherein said electron detector is a scintillator coupled to a photomultiplier.

24. The apparatus of claim 1 further including at least one secondary radiation detector within the cavity for detecting low energy gamma rays emitted by the object due to reactions with one or more elements other than nitrogen and for producing output signals representative of the concentration of said element contained within the object and means for analyzing the output signals from said secondary radiation detector to determine the position and concentration of said element contained within the object.

25. A directional channeling detector for detecting the presence and location of radiation emitted from an object comprising:

means for converting the radiation into electrons;

a channeling crystal coupled to said converting means for producing channeling radiation in response to electrons travelling through said crystal at a direction substantially parallel to a plane of the crystal lattice;

an electron detector for producing a first signal in response to an electron passing through said crystal; and

a channeling radiation detector for producing a second signal in response to channeling radiation emitted by said crystal.

26. The detector of claim 25 further including means for processing said first and second signals to produce an output signal representative of the concentration of nitrogen in the object.

27. The detector of claim 25 wherein said electron detector is a scintillator coupled to a photomultiplier tube for generating output signals in response to the conversion of radiation into electrons.

28. A method of scanning an object for nitrogen and determining the location and concentration of nitrogen in the object, comprising:

placing an object to be scanned in a cavity;

producing a thermal neutron flux within said cavity causing gamma rays to be emitted from said object in response to reactions with nitrogen contained in said object;

sensing the amount of thermal neutrons within said cavity;

adjusting the thermal neutron flux within said cavity in response to the amount of thermal neutrons;

detecting said gamma rays and producing output signals indicative of the position and energy of said gamma rays; and

analyzing said output signals to determine the concentration and position of nitrogen in the object.

29. The method of claim 28 further including generating a control signal in response to the amount of thermal neutrons within the cavity for adjusting the thermal neutron flux within said cavity.

30. An apparatus for scanning a subject to determine the distribution of nitrogen in the subject comprising:

a housing having a cavity for receiving a subject to be scanned and means for passing the subject through said cavity;

means for causing gamma rays to be emitted from the subject due to the presence of nitrogen within the subject;

at least one radiation detector having a conversion foil for converting gamma rays into electrons, a channeling crystal coupled to said conversion foil for producing channeling radiation in response to electrons travelling through said crystal substantially parallel to a plane of the crystal lattice, an electron detector for producing first signals in response to electrons passing through said crystal lattice and a solid state channeling radiation detector for producing second signals representative of the position and concentration of nitrogen contained in the subject; and

means for processing said first and second signals to determine the distribution of nitrogen in the subject.

31. The apparatus of claim 30 wherein said electron detector is a semiconductor surface barrier detector.

32. The apparatus of claim 30 wherein said electron detector is a scintillator coupled to a photomultiplier.