Method for measuring the size and velocity of spherical particles using the phase and intensity of scattered light

• US 4,986,659 A
• Filed: 10/03/1989
• Issued: 01/22/1991
• Est. Priority Date: 02/29/1988
• Status: Expired due to Term

• Current Assignee: TSI Incorporated
• Original Assignee: Aerometrics, Inc. (TSI Incorporated)
• Inventors: Bachalo, William D.
• Primary Examiner(s): Rosenberger, Richard A.
• Application Number:
  US07/416,519
• Time in Patent Office: 476 Days
• Field of Search: 356/336, 356/338, 356/343
• US Class Current: 356/336
• CPC Class Codes: G01N 15/0205 by optical means
• CPC Class Codes: G01N 2015/0216 from fluctuations of diffraction pattern
• CPC Class Codes: G01N 2015/145 by pattern of light, e.g. fringe pattern

Abstract

An improved apparatus and method for determining the change in the effective cross-section of a sample volume defined by two crossed laser beams is disclosed. A laser generation means is provided for generating a pair of coherent laser beams and means are provided to change the separation, intersection angle, and focused diameter of the beams. These beams are directed along an axis, and are caused to cross the axis at a given angle to define an interference pattern constituting a sample volume. A collection apparatus for sensing the scattering of light caused by particles, droplets, bubbles, or the like within the sample volume is provided. In the presently preferred embodiment, the collection apparatus is disposed at preferred off-axis angles including off-axis backscatter with the angle predetermined, and the angle defined by the direction of beam propagation. The collected scattered light is directed onto photo-detectors which are coupled to a signal phase determining means, for measuring the relative phase between the signals produced by each photo-detector and a signal amplitude determining means to measure the relative amplitude of the signals produced as the particle, drop, bubble, or the like passes through the sample volume. Sizing means are coupled to the signal phase and amplitude determination means for determining the size of the particle, drop, bubble, or the like from phase and amplitude changes in the received signals. Methods and apparatus are disclosed for determining the change in the effective cross-section of the sample volume due to size variations of particles passing through the interference pattern. The velocity of the particle drop, bubble, or the like is determined using well known laser Doppler anemometry techniques.

Claims

1. In an apparatus for measuring parameters associated with particles, droplets and the like employing first and second Gaussian laser beams caused to cross to establish an interference pattern forming a sample volume, a method for detecting errors due to mixed components in light scattered by said particles, droplets and the like passing through said interference pattern, comprising the steps of:

(a) generating said first and second Gaussian laser beams and directing said beams to cross at a known angle to form said sample volume;

(b) collecting said light scattered by said particles, droplets and the like passing through said sample volume and determining the phase of said scattered light;

(c) determining the size of said particles, droplets and the like from the phase of said scattered light;

(d) determining the amplitude of said scattered light and comparing said amplitude to predefined upper and lower amplitude limits for the particle size, such that if said amplitude determined is outside said limits an error is detected and said measurement is considered invalid.

2. The method as defined by claim 1, wherein said amplitude is further compared to phase angle values stored in a look-up table, said table providing a corresponding phase angle for an inputted amplitude and determines if said amplitude corresponds to a phase angle greater than 2π

.

3. The method as defined by claim 1, wherein said upper and lower amplitude limits are stored in a look-up table for each size class of said particles, droplets and the like.

4. The method as defined by claim 1, wherein said upper limit is determined by computing a theoretical value for the size class of the particle size determined and increasing the theoretical value by predetermined amount indicative of a buffer zone.

5. The method as defined by claim 4, wherein the theoretical value is computed using the Lorenz-Mie theory.

6. The method as defined by claim 4, wherein the theoretical value is computed using a geometric technique which assumes that the signal amplitude is equal to the particle diameter squared.

7. The method as defined by claim 4 wherein the predetermined amount is in the range of 0-0.25 volts.

8. The method as defined by claim 1, wherein said lower limit is determined by computing a theoretical value for the size class of the particle size determined and decreasing the theoretical value by a predetermined amount.

9. The method as defined by claim 8, wherein the theoretical value is computed using the Lorenz-Mie theory.

10. The method as defined by claim 8, wherein the theoretical value is computed using a geometric technique which assumes that the signal amplitude is equal to the particle diameter squared.

11. The method as defined by claim 8 wherein the predetermined amount is approximately one-third of the theoretical value.

12. The method as defined by claim 1, wherein said collecting step includes sensing said scattered light using two or more spaced apart photodetectors.

13. The method as defined by claim 1, wherein said mixed components comprise light reflected off of and refracted through said particles, droplets and the like.

14. In a system for measuring parameters associated with particles, droplets and the like employing laser light scattering, an apparatus for detecting errors due to mixed components in said scattering, comprising:

laser generation means for generating first and second Guassian laser beams and directing said beams to cross forming a sample volume;

collection means for collecting the scattered light due to said particles, droplets and the like passing through said sample volume, and converting said scattered light into electrical signals;

phase detection means coupled to said collection means for determining the phase and amplitude of said signals;

sizing means coupled to said phase detection means for determining the size of said particle, droplet and the like from the phase of said signals, said sizing means further comparing said amplitude to predefined upper and lower amplitude limits for the particle size, such that if said amplitude is outside said limits an error is detected and said measurement is considered invalid.

15. The apparatus as defined by claim 14, wherein said sizing means further compares said amplitude to phase angle values stored in look-up table means coupled to said sizing means, said look-up table means providing a corresponding phase angle for an inputted amplitude, and determines if said amplitude corresponds to a phase angle greater than 2π

.

16. The apparatus as defined by claim 14, wherein said upper and lower amplitude limits are stored in a look-up table for each class size of said particles, droplets and the like.

17. The apparatus as defined by claim 14, wherein said upper limit is determined by computing a theoretical value for the size class of the particle size determined and increasing the theoretical value by a predetermined amount indicative of a buffer zone.

18. The apparatus as defined by claim 17, wherein the theoretical value is computed using the Lorenz-Mie theory.

19. The apparatus as defined by claim 17, wherein the theoretical value is computed using a geometric technique which assumes that the signal amplitude is equal to the particle diameter squared.

20. The apparatus as defined by claim 17 wherein the predetermined amount is in the range of 0-0.25 volts.

21. The apparatus as defined by claim 14, wherein said lower limit is determined by computing a theoretical value for the size class of the particle size determined and decreasing the theoretical value by a predetermined amount.

22. The apparatus as defined by claim 21, wherein the theoretical value is computed using the Lorenz-Mie theory.

23. The apparatus as defined by claim 21, wherein the theoretical value is computed using a geometric technique which assumes that the signal amplitude is equal to the particle diameter squared.

24. The apparatus as defined by claim 21 wherein the predetermined amount is approximately one-third of the theoretical value.

25. The apparatus as defined by claim 14, wherein said collecting means senses said scattered light using two or more spaced apart photodetectors.

26. In an apparatus for measuring or sensing parameters associated with particles, droplets and the like employing first and second Gaussian laser beams caused to cross to establish an interference pattern forming a sample volume, a method for determining the change in the effective cross-section of said sample volume, comprising the steps of:

(a) generating said first and second Gaussian laser beams and directing said beams to cross at a known angle, said interference pattern having an apparent spacing defined as δ

;

(b) collecting the scattered signal created by said particles, droplets and the like passing through said sample volume;

(c) determining the maximum (N_max) and minimum (N_min) number of interference fringes crossed by said particles, droplets and the like, of a class of particles having the same diameter passing through said sample volume wherein N_min is the number of fringes detected to produce a signal reliable enough for later use;

(d) determining the change in the effective cross-section of said sample volume due to size variations of said particles, droplets and the like passing through said interference pattern, said change in said cross-section being defined as;

space="preserve" listing-type="equation">T(d)=δ

[N.sub.max (d).sup.2 -N.sub.min (d).sup.2 ].sup.1/2

where;

T=sample volume cross-section

d=diameter of said particle, droplet and the like

whereby the effective apparent cross-section of said sample volume is determined for a class of said particles, droplets and the like having a diameter d.

27. The method as defined by claim 26, wherein

28. The method as defined by claim 26, further including the steps of:

determining the number of particles in a size class measured; and

correcting the particle size distribution to account for the said change of cross section of said sample volume due to a non-uniform sampling of said cross-section such that;

space="preserve" listing-type="equation">n(d).sub.c =n(d)T(d.sub.max)/T(d)

where;

n(d)=number of particles measured in the size class d;

n(d)_c =corrected count for a particle, droplet and the like having diameter d;

d_max =maximum diameter of said particle, droplet and the like measured in the size distribution.

29. The method as defined by claim 28, wherein said apparatus includes collection means for collecting said scattered signal.

30. The method as defined by claim 29, wherein said collection means includes at least two photo-detectors spaced apart from one another such that said spacing of the finges formed by the scattered light is less than the distance between said first and second photo-detectors.

31. The method as defined by claim 30, wherein said collection means includes a third photo-detector spaced apart from said first and second photo-detector.

32. The method as defined by claim 31, further including the step of determining the phase shift of said scattered signal between said first and second photo-detectors and said first and third photo-detectors to determine the size range over which said particle, droplet and the like is measured.

33. In a system for measuring or sensing parameters associated with particles, droplets and the like employing laser scattering, an apparatus for determining the change in the effective cross-section of two crossed laser beams forming a sample volume, comprising:

laser generation means for generating first and second Gaussian laser beams and directing said beams to cross at a known angle (γ

), said crossed beams forming an interference pattern defining said sample volume, said interference pattern having an apparent spacing (δ

);

collection means for collecting the scattered signal created by said particle, droplet and the like passing through said sample volume;

circuit means coupled to said collection means for determining the maximum (N_max) and minimum (N_min) number of interference fringes crossed by said particles, droplets and the like, of a class of particles having the same diameter passing through said sample volume;

said circuit means further determining the change in the effective cross-section of said sample volume due to size variations of said particles, droplets and the like passing through said interference pattern, said change in said cross section being defined as;

space="preserve" listing-type="equation">T(d)=δ

[N.sub.max (d).sup.2 -N.sub.min (d).sup.2 ].sup.1/2

where;

T=sample volume cross-section;

d=diameter of said particle, droplet and the like;

whereby the effective apparent cross-section of said sample volume is determined for a class of said particles, droplets and the like having a diameter d.

34. The apparatus as defined by claim 33, wherein

35. The apparatus as defined by claim 34, wherein said circuit means utilize the number of particles in a size class measure and includes correction means for correcting said change of cross-section of said sample volume due to a non-uniform sampling of said cross-section, such that:

space="preserve" listing-type="equation">n(d).sub.c =n(d)T(d.sub.max)/T(d)

where;

n(d)=number of particles measured in the size class d;

n(d)_c =corrected count for a particle, droplet and the like having diameter d;

d_max =maximum diameter of said particle, droplet and the like measured in the size distribution.

36. The apparatus as defined by claim 35, wherein said collection means includes at least two photo-detectors spaced apart from one another such that the fringe spacing produced by the scattered light signal in the plane of the detectors is less than the distance between said first and second photodetectors.

37. The apparatus as defined by claim 36, wherein said collection means includes a third photo-detector spaced apart from said first and second photo-detector.

38. The apparatus as defined by claim 37, wherein said circuit means determines a first phase shift of said scattered signal between said first and second photodetectors and a second phase shift of said first and third photo-detectors to determine the size range over which said particle, droplet and the like is measured.

39. The apparatus as defined by claim 38, wherein said circuit means further comprises:

means for determining that the signals collected by two photodetectors are approximately 360 degrees out of phase;

a phase shifting means to shift the phase of one of the signals collected by one of the photodetectors 180 degrees such that errors due to ambiguity of overlapping signals is minimized.