Detection of explosives and other materials using resonance fluorescence, resonance absorption, and other electromagnetic processes with bremsstrahlung radiation

• US 5,420,905 A
• Filed: 10/21/1993
• Issued: 05/30/1995
• Est. Priority Date: 08/15/1990
• Status: Expired due to Term

• Current Assignee: Massachusetts Institute of Technology
• Original Assignee: Massachusetts Institute of Technology
• Inventors: Bertozzi, William
• Primary Examiner(s): Church, Craig E.
• Application Number:
  US08/140,709
• Time in Patent Office: 586 Days
• Field of Search: 378/86, 378/87, 378/88, 378/89
• US Class Current: 378/88
• CPC Class Codes: G01N 23/20091 Measuring the energy-dispersion spectrum [EDS] of diffracted radiation
• CPC Class Codes: G01N 33/0081 Containers; Packages; Bottles
• CPC Class Codes: G01V 5/222 measuring scattered radiation

Abstract

A technique for detecting explosives and other materials using resonance fluorescence, resonance absorption, and other electromagnetic processes with a continuous spectrum of photons is disclosed. The method is particularly attractive as a way to detect explosives at airports and other transporation terminals. According to one aspect of the invention, bremsstrahlung or other continuous-spectrum photon radiation in the appropriate energy ranges is made incident on a target (e.g., a piece of luggage or other container) to resonantly excite the atoms of the target. In one embodiment, the energies of the photons scattered directly from the target are detected and measured. These energies are characteristic of the nuclear species excited in the target, and thus the concentrations of these elements in the target can be determined. A high concentration of nitrogen and oxygen with a low concentration of carbon indicates practically without fail an explosive material. In another embodiment, the energies of photons resonantly scattered from reference scatterers composed substantially of nuclear species of interest and located downstream from the target are detected and measured. The abundance of photons of energies corresponding to nuclear species of interest detected in this embodiment is inversely related to the abundance of the species in the target. In another aspect of the invention, electromagnetic processes occuring in the target as the photon beam passes through the target, in particular, Compton scattering and pair production, are detected to create three-dimensional images of the spatial distribution of the density and the atomic number or charge of the target. All four detection schemes of the invention are compatible and can be used individually or in combination to increase detectability of species in various situations.

Claims

1. A method for characterizing material composition of a target comprising:

resonantly exciting nuclei of the target with a continuous spectrum of photons,

resonantly exciting nuclei of one or more reference scatterers with the photons transmitted through the target, each said reference scatterer comprising one or more nuclear species of interest,

measuring the intensity of photons at energies of interest scattered from each said reference scatterer in a direction or directions, said energies of interest for each reference scatterer corresponding to the spacings between the quantized energy states of the nuclear species of interest of which the reference scatterer is comprised,

estimating the abundance of each nuclear species of interest in the target from the measured intensity of photons scattered from the reference scatterer or scatterers comprising the nuclear species,

measuring the intensity of photons at energies of interest produced in and emitted from the target in a direction or directions, said energies of interest corresponding to pair production with subsequent positive electron annihilation in the target, and

estimating the spatial distribution of the quantity DZ² /A, where D is density, Z is nuclear charge, and A is number of nucleons, in the target from the measured intensity of photons produced by pair production emitted from the target.

2. The method of claim 1 further comprising:

measuring the intensity of photons at energies of interest scattered from the target in a direction or directions, said energies of interest corresponding to the spacings between the quantized energy states of nuclear species of interest, said nuclear species of interest being the same as or different from the nuclear species of which the reference scatterers are comprised, and

estimating the abundance of nuclear species of interest in the target from the measured intensity of photons scattered from the target which correspond to nuclear species of interest.

3. A device for characterizing material composition of a target comprising:

a shielded source of a continuous spectrum of photons;

means for making the photons incident on said target;

detecting apparatus comprising an array or arrays of individual detectors for capturing, measuring, counting and recording the energies of photons produced by pair production in said target; and

computing apparatus for accepting data from said detecting apparatus and using this data to characterize the material properties of the target and further comprising one or more reference resonance scatterers positioned such that photons transmitted through the target will be incident on said resonance scatterers and one or more detecting apparatuses each comprising an array of individual detectors for capturing, measuring, counting, and recording the energies of photons scattered from said reference scatterers.

4. The device of claim 3 further comprising detecting appraratus for capturing, measuring, counting, and recording the energies of photons resonantly scattered from said target.

5. The device of claim 3 further comprising detecting apparatus for capturing, measuring, counting, and recording the energies of photons Compton scattered from said target.

6. The device of claim 5 further comprising detecting appraratus for capturing, measuring, counting, and recording the energies of photons resonantly scattered from said target.