Method for operating a chemical and/or physical process by means of a hierarchical fluid injection system

• US 6,333,019 B1
• Filed: 04/29/1999
• Issued: 12/25/2001
• Est. Priority Date: 04/29/1999
• Status: Expired due to Term

• Current Assignee: Marc-Olivier Coppens
• Original Assignee: Marc-Olivier Coppens
• Inventors: Coppens, Marc-Olivier
• Primary Examiner(s): LANGEL, WAYNE A
• Application Number:
  US09/301,971
• Time in Patent Office: 971 Days
• Field of Search: 423/659, 423/DIG.16, 232/93.R, 233/13.FB, 261/20, 261/DIG.70, 261/DIG.80, 518/728
• US Class Current: 423/659
• CPC Class Codes: B01F 25/40 Static mixers colloid-mills B02C; mixing valves F16K11/00
• CPC Class Codes: B01F 25/41 Mixers of the fractal type
• CPC Class Codes: B01F 35/7182 with means for feeding the material with a fractal or tree-type distribution in a surface
• CPC Class Codes: B01J 10/002 carried out in foam, aerosol or bubbles
• CPC Class Codes: B01J 2208/00725 Mathematical modelling
• CPC Class Codes: B01J 8/1827 the fluidising gas being a reactant
• CPC Class Codes: B01J 8/22 gas being introduced into the liquid
• CPC Class Codes: Y10S 261/70 Sewage aerators; diffusers
• CPC Class Codes: Y10S 261/71 Sewage aerators; rotating
• CPC Class Codes: Y10S 423/16 Fluidization

Abstract

The invention relates to injection of fluids (gas, liquid, suspension or other mixtures) in a controlled typically uniform way within a vessel containing another fluid or fluidized medium. Said injection device consists of pipes or channels that are connected in a hierarchical fashion so that the fluid entering a first channel is divided into channels of the same or different diameter and length, each or some of which are further divided into channels of the same or different diameter and length, and so on. The injection system can also consist of combinations of such tree-like or fractal-like elements, embedded in the plane or in space.

The embodiment depends upon the nature of the fluids and the application. The invention can be used for gas/solid fluidized bed and a gas/liquid and other processes. A typical application is the reduction and uniformization or otherwise control of bubble sizes to optimize the operation of fluidized bed, slurry and gas/liquid reactors.

Claims

1. Method for operating a multi-phase process that is chemical, physical, or both, in a vessel containing at least two different phases selected from the group consisting of a liquid phase, a gas phase and a solid phase, inside which vessel a fluid is distributed through a hierarchical network of channels comprising parent and child generations of channel formations, wherein substantially each channel in a parent generation is divided into N channels of a child generation, wherein each channel of said child generation may in turn be a parent for channels in a successive child generation, which network terminates in channel exits, such that said fluid is discharged from the channel exits substantially uniformly throughout the vessel volume.

2. Method according to claim 1 in which said network is a self-affine network of channels, wherein each of the channels in the parent generation has a diameter d_j and a length l_j, and each of the channels in the child generation has a diameter d_j+1 and a length l_j+1, wherein at least one of the ratios d_j/d_j+1 and l_j/l_j+1 is substantially constant for channels of successive generations running in parallel direction.

3. Method according to claim 2 wherein the diameters or the lengths of channels in successive generations of said network, or both, are related to N by at least one of the following relationships:

4. Method according to claim 2, wherein said self-affine network is a self-similar network, in which the ratios d_j/d_j+1 and l_j/l_j+1 are both substantially constant for channels of successive generations independent of their direction.

5. Method according to claim 1, in which said multi-phase process is selected from a group consisting of a fluidized bed process, a slurry process, an absorption process, a gas/liquid bubble column process, and an aeration process.

6. Method for operating a process that is chemical, physical, or both, in a vessel containing at least two different phases selected from the group consisting of a liquid phase, a gas phase and a solid phase, throughout which vessel a fluid is distributed through a hierarchical network of channels comprising parent and child generations of channel formations, wherein substantially each channel in a parent generation is divided into N channels of the child generation, wherein each channel of said child generation may in turn be a parent for channels in a successive child generation, which network terminates in channel exits, such that said fluid is discharged from the channel exits substantially uniformly throughout the vessel volume, wherein said network is a self-affine network of channels, wherein each of the channels in the parent generation has a diameter d_j and a length l_j, and each of the channels in the child generation has a diameter d_j+1 and a length l₊₁, wherein at least one of the ratios d_j/d_j+1 and l_j/l_j+1 is substantially constant for channels of successive generations running in parallel direction, wherein the ratio of lengths of channels in successive generations of said network is related to N by the formula, N=(l_j/l_j+1)^D, wherein D is between 2 and 3.

7. Method according to claim 6, wherein the ratio of diameters of channels in successive generations of said network is related to N by the formula, N=(d_j/d_j+1)^Δ

, wherein Δ

represents an integer or a real positive number.

8. Method according to claim 6, wherein said self-affine network is a self-similar network in which the ratios d_j/d_j+1 and l_j/l_j+1 are both substantially constant for channels of successive generations, independent of their direction.

9. Method for scaling up a multi-phase process that is chemical, physical, or both, and that is carried out in a vessel containing at least two different phases selected from the group consisting of a liquid phase, a gas phase and a solid phase, comprising the steps of:

building a small scale vessel;

distributing a fluid through a hierarchical network of channels comprising parent and child generations of channel formations, wherein substantially each channel in a parent generation is divided into about N channels of the child generation, wherein each of the channels in the parent generation has a diameter d_j and a length l_j and each of the channels in a child generation has a diameter d_j+1 and a length l_j+1, which network terminates in channel exits, such that said fluid is discharged from the channel exits substantially uniformly throughout the vessel volume;

determining optimal geometry and optimal values for the parameters, N, Δ and

D, wherein the diameters or the lengths of channels in successive generations of said network, or both, are related to N by at least one of the following relationships;

N=(d_j/d_j+1) Δ and

N=(l_j/l_j+1)^D, wherein Δ and

D each represents an integer or a real positive number; and

subsequently building a large scale vessel having substantially the same geometry and parameters as the small scale vessel, and having a larger number of generations than the small scale vessel.