X-ray backscatter imaging of nuclear materials

• US 8,848,871 B2
• Filed: 11/03/2011
• Issued: 09/30/2014
• Est. Priority Date: 11/04/2010
• Status: Active Grant

• Current Assignee: UT-Battelle LLC
• Original Assignee: UT-Battelle LLC
• Inventors: Hollenbach, Daniel F., Ott, Larry J., Shedlock, Daniel, Chapman, Jeffrey Allen, Gunning, John E.
• Primary Examiner(s): Ho, Allen C.
• Application Number:
  US13/288,168
• Publication Number:
  US 20120114102A1
• Time in Patent Office: 1,062 Days
• Field of Search: 378 88- 90
• US Class Current: 378/87
• CPC Class Codes: G01N 23/203 Measuring back scattering

Abstract

The energy of an X-ray beam and critical depth are selected to detect structural discontinuities in a material having an atomic number Z of 57 or greater. The critical depth is selected by adjusting the geometry of a collimator that blocks backscattered radiation so that backscattered X-ray originating from a depth less than the critical depth is not detected. Structures of Lanthanides and Actinides, including nuclear fuel rod materials, can be inspected for structural discontinuities such as gaps, cracks, and chipping employing the backscattered X-ray.

Claims

1. A method of imaging a high-Z material-including structure by X-ray backscatter imaging, said method comprising:

irradiating a target including a high-Z material-including structure with an incident X-ray radiation from an X-ray source, said high-Z material-including structure including at least one element having an atomic number of at least 57;

detecting a backscattered X-ray radiation from said target with at least one detector-collimator assembly positioned to block a fraction of said backscattered X-ray radiation originating at depths less than a critical depth from a top surface of said target; and

constructing an image of said target employing at least data collected at said at least one detector-collimator assembly, said image including information on structural discontinuity of said high-Z material-including structure.

2. The method of claim 1, wherein said at least one element is selected from Lanthanides and Actinides.

3. The method of claim 1, wherein said at least one element is a fissile material.

4. The method of claim 1, wherein said high-Z material-including structure includes an oxide, a nitride, a carbide, a fluoride, or a boride of said at least one element.

5. The method of claim 1, wherein said high-Z material-including structure includes a nuclear fuel material that is encased in a cladding.

6. The method of claim 5, wherein said high-Z material—

including structure includes UO₂.

7. The method of claim 5, wherein said high-Z material-including structure includes a manufactured nuclear fuel rod in which atomic ratio of fissile atoms to fission products is greater than 5:

1.

8. The method of claim 5, wherein said high-Z material-including structure includes a spent nuclear fuel rod that has been removed from a nuclear reactor.

9. The method of claim 1, wherein said target includes a stack of said high-Z material-including structure and a cladding that encloses said high-Z material-including structure, and wherein said critical depth is within said high-Z material-including structure during said irradiating and said detecting.

10. The method of claim 1, further comprising scanning different areas of said target with said incident X-ray radiation by providing a relative movement between said target and said X-ray source.

11. The method of claim 10, wherein a distance between said target and said at least one detector-collimator assembly is maintained at a constant value during said scanning.

12. The method of claim 10, wherein said relative movement is provided continuously while said target is continuously irradiated with said incident X-ray radiation.

13. The method of claim 10, wherein said relative movement is provided between each sequential irradiation of different areas of said target with said incident X-ray radiation.

14. The method of claim 10, wherein said relative movement is provided by maintaining said target stationary and moving said X-ray source and said at least one detector-collimator assembly.

15. The method of claim 10, wherein said X-ray source and said at least one detector-collimator assembly moves at the same rate of movement in a same direction throughout said relative movement.

16. The method of claim 15, wherein said target is a nuclear fuel rod, and said relative movement is provided by moving said X-ray source and said at least one detector-collimator along a lengthwise direction of said nuclear fuel rod.

17. The method of claim 10, wherein said relative movement is provided by maintaining said X-ray source and said at least one detector-collimator assembly stationary while moving said target.

18. The method of claim 1, wherein said incident X-ray radiation includes photons having energy in a range from 150 keV to 800 keV.

19. The method of claim 1, wherein said at least one element having an atomic number of at least 57 is an Actinide, and said incident X-ray radiation includes photons having energy in a range from 500 keV to 700 keV.

20. The method of claim 19, wherein said Actinide is uranium, and said high-Z material-including structure includes UO₂.

21. The method of claim 1, wherein said image of said target is constructed by processing said data collected at said at least one detector-collimator assembly with a computing device.

22. The method of claim 1, further comprising

changing a distance between said at least one detector-collimator assembly and said target, wherein said at least one detector-collimator assembly becomes positioned to block of another fraction of said backscattered X-ray radiation originating at depths less than a second critical depth from said top surface of said target, wherein said second critical depth is different from said critical depth;

and

irradiating said target with said incident X-ray radiation from said X-ray source while said changed distance is maintained.

23. The method of claim 22, further comprising constructing a second image of said target from additional data collected at said at least one detector-collimator assembly while said changed distance is maintained, said second image including additional information on structural discontinuity of said high-Z material-including structure.

24. The method of claim 23, wherein said image and said second image are 2-dimensional images, and said method further comprises constructing a 3-dimensional image of said target from a set of images including at least said image and said second image.

25. The method of claim 22, wherein said image is a 3-dimensional image that is constructed from said data and additional data collected at said at least one detector-collimator assembly while said changed distance is maintained.