Two-dimensional detection system for neutron radiation in the field of neutron scattering spectrometry

• US 9,040,934 B2
• Filed: 04/28/2014
• Issued: 05/26/2015
• Est. Priority Date: 03/10/2005
• Status: Expired due to Fees

• Current Assignee: Commissariat a L'Energie Atomique (AES Corporation), Centre National De La Recherche Scientifique
• Original Assignee: Commissariat a L'Energie Atomique (AES Corporation), Centre National De La Recherche Scientifique
• Inventors: Baroni, Patrick Francois, Noirez, Laurence Marie
• Primary Examiner(s): Porta, David
• Assistant Examiner(s): VU, MINDY D
• Application Number:
  US14/262,914
• Publication Number:
  US 20140231661A1
• Time in Patent Office: 393 Days
• Field of Search: 250/390.11
• US Class Current: 250/390.11
• CPC Class Codes: G01N 23/2073 using neutron detectors neutron spectrometry G01T3/00
• CPC Class Codes: G01T 3/00 Measuring neutron radiation G01T5/00 takes precedence
• CPC Class Codes: G01T 3/001 Spectrometry
• CPC Class Codes: G01T 3/06 with scintillation detectors
• CPC Class Codes: G01T 3/065 Spectrometry

Abstract

This invention relates to a two-dimensional detection system for neutron radiation comprising a means (1) for emitting a neutron beam (10), a support means (2) adapted for receiving a sample (3), a photoemission means (5) adapted for being activated by a neutron radiation, a cooled low light level charge-coupled detection device (7). The emission means (1) emits a monochromatic neutron beam (10). The system further comprises a filter means (4), the filter means (4) being located between the support means (2) and the photoemission means (5) and being adapted for trapping at least a substantial part of the monochromatic neutron beam transmitted (12) by the sample (3), and an amplification means (6) located upstream the charge-coupled detection device (7) and coupled with the charge-coupled detection device (7).

Claims

1. Two-dimensional neutron detection system for neutron scattering comprising

(a) an emission means configured for emitting a monochromatic neutron beam,

(b) a support means for receiving a sample, arranged in the trajectory of the monochromatic neutron beam;

(c) a photoemission means for activation by neutrons, arranged in the trajectory of the monochromatic neutron beam after the (b) support means, wherein (c) the photoemission means comprises a lithium-based scintillator which emits alpha radiation originating from a single nuclear reaction;

(d) a filter means, said filter means being located between (b) the support means and the (c) photoemission means and being adapted for trapping the entire monochromatic neutron beam transmitted by the sample such that scattered neutrons from the sample reach and activate the (c) photoemission means; and

wherein the (c) photoemission means detects only the number of neutrons scattered by the sample and is in the direct path of the (a) emission means and (d) filter means;

(e) a cooled low light level charge-coupled detection device,

(f) an amplification means located upstream of (e) the charge-coupled detection device and coupled with (e) the charge-coupled detection device, said (f) amplification means and said (e) charge-coupled detection device being surrounded by a shield for stopping gamma radiation; and

wherein

said (c) photoemission means, said (f) amplification means, and said (e) charge-coupled detection device are enclosed in a box designed such that no light radiation other than that emitted by the (c) photoemission means can penetrate inside, said (c) photoemission means forming an inlet wall of the box, and said (e) charge-coupled detection device coupled with said (f) amplification forming an outlet wall of the box, wherein the outlet wall is adjacent to the inlet wall.

2. Two-dimensional neutron detection system for neutron scattering according to claim 1, wherein the lithium-based scintillator is a composite material based on lithium sulphide.

3. Two-dimensional neutron detection system for neutron scattering according to claim 1, wherein the lithium-based scintillator is a composite material based on lithium fluoride.

4. Two-dimensional neutron detection system for neutron scattering according to claim 1,

wherein

(c) the photoemission means is in the form of a plate with a length of between 5 and 100 cm, a width of between 5 and 100 cm and a thickness of less than or equal to 1.2 mm.

5. Two-dimensional neutron detection system for neutron scattering according to claim 1, wherein (c) the photoemission means is plane.

6. Two-dimensional neutron detection system for neutron scattering according to claim 1, wherein (c) the photoemission means is curved, defined by a portion of cylinder delimited by a plane with dimensions varying from 5 to 100 cm in length and in width.

7. Two-dimensional neutron detection system for neutron scattering according to claim 1, wherein (c) the photoemission means is curved, defined by a portion of sphere.

8. Two-dimensional neutron detection system for neutron scattering according to claim 1, wherein (c) the photoemission means is lined with a surface opaque to light and transparent to neutron scattering, and located on the inlet of (c) the photoemission means.

9. Two-dimensional neutron detection system for neutron scattering according to claim 8, wherein the opaque surface is formed from a rigid material adapted for holding (c) the photoemission means in place.

10. Two-dimensional neutron detection system for neutron scattering according to claim 8, wherein the opaque surface is an aluminum plate.

11. Two-dimensional neutron detection system for neutron scattering according to claim 1, wherein (e) the charge-coupled detection device enables coding on at least 12 bits.

12. Two-dimensional neutron detection system for neutron scattering according to claim 11, wherein (e) the charge-coupled detection device enables coding on at least 16 bits.

13. Two-dimensional neutron detection system for neutron scattering according to claim 1, wherein (e) the charge-coupled detection device is a camera adapted for variable pause times.

14. Two-dimensional neutron detection system for neutron scattering according to claim 1,

wherein

the system further comprises a protection means capable of reducing the influence of parasite radiation between the (b) support means for the sample and (c) the photoemission means.

15. Two-dimensional neutron detection system for neutron scattering according to claim 14, wherein the protection means is a conical or pyramid shaped element, having (c) the photoemission means as its base and being located between (b) the support means for the sample and (c) the photoemission means.

16. Two-dimensional neutron detection system for neutron scattering according to claim 14, wherein the protection means is a casing comprising a cylindrical part and a tapered end part, and surrounding the box.

17. Two-dimensional neutron detection system for neutron scattering according to claim 14, wherein the protection means includes sidewalls adapted for absorbing parasite radiation not originating from the sample.

18. Two-dimensional neutron detection system for neutron scattering according to claim 14, wherein the protection means contains an inert gas or a primary vacuum.

19. Two-dimensional neutron detection system for neutron scattering according to claim 18, wherein the inert gas is helium.

20. Two-dimensional neutron detection system for neutron scattering according to claim 18, wherein the inert gas is argon.

21. Two-dimensional neutron detection system for neutron scattering according to claim 18, wherein the inert gas is nitrogen.

22. Two-dimensional neutron detection system for neutron scattering according to claim 1, wherein the box comprises inside walls adapted for absorbing neutron and gamma radiation.

23. Two-dimensional neutron detection system for neutron scattering according to claim 1, wherein the system further comprises a minor adapted for reflecting only light radiation emitted by (c) the photoemission means towards (f) the amplification means.

24. Two-dimensional neutron detection system for neutron scattering according to claim 23, wherein the minor is made from aluminized quartz and is less than or equal to 10 mm thick.

25. Two-dimensional neutron detection system for neutron scattering according to claim 23, wherein the minor is plane.

26. Two-dimensional neutron detection system for neutron scattering according to claim 23, wherein the minor is curved.

27. Two-dimensional neutron detection system for neutron scattering according to claim 1, wherein the system further comprises a means for absorbing neutron and gamma radiation, this absorption means being arranged at the outlet of (c) the photoemission means.

28. Two-dimensional neutron detection system for neutron scattering according to claim 1, wherein the shield is a metal with a thickness and a density such that the product of the thickness and the density is greater than or equal to 34.

29. Two-dimensional neutron detection system for neutron scattering according to claim 1, wherein the shield is made of tungsten with a thickness of about 2 cm.

30. Two-dimensional neutron detection system for neutron scattering according to claim 1, wherein the system further comprises a collimation device arranged between (a) the emission means and (b) the support means, and outputting an output neutron beam with a diameter of between 0.5 and 15 mm.

31. Two-dimensional neutron detection system for neutron scattering according to claim 1 wherein (c) the photoemission means device detects only the number of neutrons scattered by a sample at wide diffusion angles.

32. Two-dimensional neutron detection system for neutron scattering according to claim 1, wherein said two-dimensional neutron detection system consists essentially of:

(a) an emission means configured for emitting a monochromatic neutron beam,

(b) a support means for receiving a sample, arranged in the trajectory of the monochromatic neutron beam;

(c) a photoemission means for activation by neutrons, arranged in the trajectory of the monochromatic neutron beam after the (b) support means, wherein (c) the photoemission means comprises a lithium-based scintillator which emits alpha radiation originating from a single nuclear reaction;

(d) a filter means, said filter means being located between (b) the support means and the (c) photoemission means and being adapted for trapping the entire monochromatic neutron beam transmitted by the sample such that scattered neutrons from the sample reach and activate the (c) photoemission means; and

wherein the (c) photoemission means detects only the number of neutrons scattered by the sample and is in the direct path of the (a) emission means and (d) filter means;

(e) a cooled low light level charge-coupled detection device,

(f) an amplification means located upstream of (e) the charge-coupled detection device and coupled with (e) the charge-coupled detection device, said (f) amplification means and said (e) charge-coupled detection device being surrounded by a shield for stopping gamma radiation; and

wherein

said (c) photoemission means, said (f) amplification means, and said (e) charge-coupled detection device are enclosed in a box designed such that no light radiation other than that emitted by the (c) photoemission means can penetrate inside, said (c) photoemission means forming an inlet wall of the box, and said (e) charge-coupled detection device coupled with said (f) amplification forming an outlet wall of the box, wherein the outlet wall is adjacent to the inlet wall.