Precursor formulation for battery active materials synthesis
First Claim
1. A chemical composition, comprising:
- a water miscible solution comprising a first battery active metal cation, a second batter active metal cation, and reactive anions, wherein the first battery active metal cation is lithium; and
a water miscible organic material selected from the group consisting of hexamethylene tetramine, carbohydrazide, oxalic acid dihydrazide, malonic acid dihydrazide, maleic hydrazide, diformyl hydrazide, tetraformal trisazine, and combinations and derivatives thereof, wherein the water miscible organic material is between about 0.1 weight percent and about 10 weight percent of the chemical composition.
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Abstract
Compositions and methods of forming battery active materials are provided. A solution of battery active metal cations and reactive anions may be blended with a fuel to yield a precursor mixture usable for synthesizing a battery active material for deposition onto a substrate. The battery active metal cations include lithium, manganese, cobalt, nickel, iron, vanadium, and the like. Reactive anions include nitrate, acetate, citrate, tartrate, maleate, azide, amide, and other lower carboxylates. Suitable fuels, which may be water miscible, may include amino compounds. Alcohols and sugars may be added to adjust carbon content and fuel combustion characteristics. An exothermic reaction is performed to convert the metals into battery active oxides.
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Citations
17 Claims
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1. A chemical composition, comprising:
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a water miscible solution comprising a first battery active metal cation, a second batter active metal cation, and reactive anions, wherein the first battery active metal cation is lithium; and a water miscible organic material selected from the group consisting of hexamethylene tetramine, carbohydrazide, oxalic acid dihydrazide, malonic acid dihydrazide, maleic hydrazide, diformyl hydrazide, tetraformal trisazine, and combinations and derivatives thereof, wherein the water miscible organic material is between about 0.1 weight percent and about 10 weight percent of the chemical composition. - View Dependent Claims (2, 3, 4, 5, 6, 7, 8, 9, 10, 11)
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12. A chemical composition, comprising:
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a water miscible solution comprising a first battery active metal cation, a second battery active metal cation, and reactive anions, wherein the first battery active metal cation is lithium, wherein the second battery active metal cation is selected from the group consisting of nickel, cobalt, and manganese; and a water miscible organic material selected from the group consisting of hexamethylene tetramine, carbohydrazide, oxalic acid dihydrazide, malonic acid dihydrazide, maleic hydrazide, diformyl hydrazide, tetraformal trisazine, and combinations and derivatives thereof, wherein the water miscible organic material is between about 0.1 weight percent and about 10 weight percent of the chemical composition. - View Dependent Claims (13, 14, 15, 16, 17)
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Specification