Neutron detector with interblended liquid scintillator

• US 9,568,623 B2
• Filed: 11/18/2014
• Issued: 02/14/2017
• Est. Priority Date: 11/18/2014
• Status: Expired due to Fees

• Current Assignee: Palo Alto Research Center, Inc. (Xerox Holdings Corp.)
• Original Assignee: Palo Alto Research Center, Inc. (Xerox Holdings Corp.)
• Inventors: Sahu, Saroj Kumar, Eldershaw, Craig, Sheridan, Martin
• Primary Examiner(s): Bryant, Casey
• Application Number:
  US14/547,092
• Publication Number:
  US 20160139280A1
• Time in Patent Office: 819 Days
• US Class Current: 1/1
• CPC Class Codes: G01T 3/06 with scintillation detectors

Abstract

A neutron detector that utilizes cells in which a liquid scintillator is contained in elongated detector tubes, with photo-detectors disposed at each end of the tube to measure scintillation light generated by incident neutrons. The liquid scintillator is an interblended mixture including an ionic liquid blended with a scintillation enhancer and/or a moderator and/or a controlled optical attenuator. A longitudinal position of an incident neutron is determined by the magnitudes of the scintillation light portions arriving at each photo-detector, which are proportional to the distances between the neutron interaction point and the photo-detectors. The cells are arranged in a closely-spaced parallel planar array to facilitate determining incident neutron location in two dimensions. A detector system utilizes a first detector array to detect fast neutrons, a thermalizer (e.g., polyethylene) to convert fast incident neutrons to thermal neutrons, and a second detector array to detect the thermal neutrons.

Claims

1. A neutron detector cell comprising:

an elongated detector tube having a first end and an opposing second end and including a peripheral wall defining an enclosed channel,

a liquid scintillator disposed in the elongated channel, said liquid scintillator including an ionic liquid blended with a controlled optical attenuator and at least one of a scintillation enhancer and a moderator such that the liquid scintillator is configured to generate a light pulse at an interaction point in response to an incident neutron, and configured such that light transmitted along the elongated detector tube from said light pulse is attenuated by an amount that is inversely proportional to a distance traveled from the interaction point along the elongated detector tube;

a first photo-detector optically coupled to the first end of said elongated detector tube, said first photo-detector configured to detect a first portion of said light pulse that is transmitted from said interaction point through said liquid scintillator to the first end, and to generate a first detection signal including a first light magnitude value indicating a first light amount of said first portion; and

a second photo-detector optically coupled to the second end of said elongated detector tube, said second photo-detector configured to detect a second portion of said light pulse transmitted from said interaction point through said liquid scintillator to the second end, and to generate a second detection signal including a second light magnitude value indicating a second light amount of said second portion, whereby a longitudinal location of said light pulse along said elongated detector tube is determinable by a difference between said first and second light magnitude values.

2. The neutron detector cell of claim 1, wherein the ionic liquid of the liquid scintillator comprises one or more anions derived from the group including derived from the group including [BF₄]⁻

, [PF₆]⁻

, [CF₃SO₂NSO₂CF₃]⁻

, [CF₃SO₃]⁻

, and [N(CN)₂]⁻

, and one or more cations derived from the group including imidazolium, pyridinium, pyrimidinum, pyrazinium, pyrazolium, piperdinium and pyrrolidinium.

3. The neutron detector cell of claim 2, wherein the liquid scintillator comprises said ionic liquid blended with at least one of Athracene, an organic scintillator and inorganic scintillator.

4. The neutron detector cell of claim 2, wherein the liquid scintillator comprises said ionic liquid blended with at least one of Lithium and Boron.

5. The neutron detector cell of claim 2, wherein the liquid scintillator comprises said ionic liquid blended with at least one organic dye.

6. The neutron detector of claim 1, wherein the ionic liquid comprises a Room Temperature Ionic Liquid (RTIL).

7. The neutron detector cell of claim 6, wherein the liquid scintillator consists essentially of said RTIL blended with Anthracene.

8. The neutron detector cell of claim 6, wherein the liquid scintillator consists essentially of said RTIL blended with Lithium isotopes ⁶Li, Boron isotopes ¹⁰B and an organic dye.

9. The neutron detector cell of claim 6, wherein the liquid scintillator consists essentially of said RTIL blended with Lithium isotopes ⁶Li, Boron isotopes ¹⁰B, an organic dye and Anthracene.

10. The neutron detector cell of claim 1, further comprising a tapered light guide disposed between the first end of said detector tube and said first photo-detector.

11. The neutron detector cell of claim 1,

wherein the peripheral wall of the detector tube comprises one of plastic and glass, and

wherein the neutron detector cell further comprises:

a reflective layer comprising a reflective material disposed on an outside surface of the peripheral wall; and

a light-sealing layer comprising a material that is opaque to black light disposed on an outside surface of the reflective layer.

12. A neutron detector cell comprising:

an elongated detector tube having a first end and an opposing second end and including a peripheral wall defining an enclosed channel,

a liquid scintillator disposed in the elongated channel, said liquid scintillator including an ionic liquid blended with at least one of a scintillation enhancer, a moderator and a controlled optical attenuator;

a first photo-detector optically coupled to the first end of said detector tube, said first photo-detector configured to detect a light pulse generated by said liquid scintillator, and to generate a first detection signal including a first light magnitude value indicating a first portion of said light pulse arriving at said first end of said detector tube; and

a second photo-detector optically coupled to the second end of said detector tube, said second photo-detector configured to detect said light pulse and to generate a second detection signal including a second light magnitude value indicating a second portion of said light pulse arriving at said second end of said detector tube,

wherein the ionic liquid of the liquid scintillator comprises one or more anions derived from the group including derived from the group including [BF₄]⁻

, [PF₆]⁻

, [CF₃SO₂NSO₂CF₃]⁻

, [CF₃SO₃]⁻

, and [N(CN)₂]⁻

, and one or more cations derived from the group including imidazolium, pyridinium, pyrimidinum, pyrazinium, pyrazolium, piperdinium and pyrrolidinium blended with at least one organic dye, and

wherein the organic dye comprises an anthraquinone-based organic dye.

13. A neutron detector cell comprising:

an elongated detector tube having a first end and an opposing second end and including a peripheral wall defining an enclosed channel,

a liquid scintillator disposed in the elongated channel, said liquid scintillator including an ionic liquid blended with at least one of a scintillation enhancer, a moderator and a controlled optical attenuator;

a first photo-detector optically coupled to the first end of said detector tube, said first photo-detector configured to detect a light pulse generated by said liquid scintillator, and to generate a first detection signal including a first light magnitude value indicating a first portion of said light pulse arriving at said first end of said detector tube; and

a second photo-detector optically coupled to the second end of said detector tube, said second photo-detector configured to detect said light pulse and to generate a second detection signal including a second light magnitude value indicating a second portion of said light pulse arriving at said second end of said detector tube,

wherein the ionic liquid comprises a Room Temperature Ionic Liquid (RTIL), and

wherein the liquid scintillator consists essentially of said RTIL blended with Lithium isotopes ⁶Li and Boron isotopes ¹⁰B.